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arxiv: 1405.4101 · v1 · pith:BMGCXEVLnew · submitted 2014-05-16 · ❄️ cond-mat.supr-con · cond-mat.mes-hall· cond-mat.mtrl-sci· cond-mat.str-el

Multiscale distribution of oxygen puddles in 1/8 doped YBa2Cu3O6.67

classification ❄️ cond-mat.supr-con cond-mat.mes-hallcond-mat.mtrl-scicond-mat.str-el
keywords beamdistributionoxygenx-raydiffractiondopantsinhomogeneitylack
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Despite intensive research a physical explanation of high Tc superconductors remains elusive. One reason for this is that these materials have generally a very complex structure making useless theoretical models for a homogeneous system. Little is known on the control of the critical temperature by the space disposition of defects because of lack of suitable experimental probes. X-ray diffraction and neutron scattering experiments used to investigate y oxygen dopants in YBa2Cu3O 6+y lack of spatial resolution. Here we report the spatial imaging of dopants distribution in-homogeneity in YBa2Cu3O6.67 using scanning nano X-ray diffraction. By changing the X-ray beam size from 1 micron to 300 nm of diameter, the lattice inhomogeneity increases. The ordered oxygen puddles size distribution vary between 6-8 nm using 1x1 {\mu}m2 beam, while it is between 5-12 nm with a fat tail using the 300x300 nm2 beam. The increased inhomogeneity at the nanoscale points toward an intrinsic granular complexity.

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