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Metal-organic Frameworks: Possible New Two-Dimensional Magnetic and Topological materials

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arxiv 2011.07088 v1 pith:ZE7RLO2O submitted 2020-11-13 cond-mat.mtrl-sci physics.comp-ph

Metal-organic Frameworks: Possible New Two-Dimensional Magnetic and Topological materials

classification cond-mat.mtrl-sci physics.comp-ph
keywords magneticmaterialsframeworksmetal-organicmofspropertiestopologicaltwo-dimensional
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Finding new two-dimensional (2D) materials with novel quantum properties is highly desirable for technological innovations. In this work, we studied a series of metal-organic frameworks (MOFs) with different metal cores and discovered various attractive properties, such as room-temperature magnetic ordering, strong perpendicular magnetic anisotropy, huge topological band gap (>200meV), and excellent spin-filtering performance. As many MOFs have been successfully synthesized in experiments, our results suggest realistic new 2D functional materials for the design of spintronic nanodevices.

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