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arxiv: 2306.12493 · v2 · pith:NECEN2EPnew · submitted 2023-06-21 · ❄️ cond-mat.supr-con · cond-mat.mes-hall· cond-mat.mtrl-sci· cond-mat.str-el

Self-doped flat band and spin-triplet superconductivity in monolayer 1T-TaSe_(2-x)Te_(x)

classification ❄️ cond-mat.supr-con cond-mat.mes-hallcond-mat.mtrl-scicond-mat.str-el
keywords flatbandmagneticsuperconductingtaseleadingmetalmonolayer
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Two-dimensional van der Waals materials have become an established platform to engineer flat bands which can lead to strongly-correlated emergent phenomena. In particular, the family of Ta dichalcogenides in the 1\textit{T} phase presents a star-of-David charge density wave that creates a flat band at the Fermi level. For TaS$_2$ and TaSe$_2$ this flat band is at half filling leading to a magnetic insulating phase. In this work, we theoretically demonstrate that ligand substitution in the TaSe$_{2-x}$Te$_x$ system produces a transition from the magnetic insulator to a non-magnetic metal in which the flat band gets doped away from half-filling. For $x\in[{0.846},{1.231}]$ the spin-polarized flat band is self-doped and the system becomes a magnetic metal. In this regime, we show that attractive interactions promote three different spin-triplet superconducting phases as a function of $x$, corresponding to a nodal f-wave and two topologically-different chiral p-wave superconducting phases. Our results establish monolayer TaSe$_{2-x}$Te$_{x}$ as a promising platform for correlated flat band physics leading to unconventional superconducting states.

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