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Exciton diffusion in WSe2 monolayers embedded in a van der Waals heterostructure

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arxiv 1802.09201 v1 pith:MKG7IHWZ submitted 2018-02-26 cond-mat.mes-hall cond-mat.mtrl-sci

Exciton diffusion in WSe2 monolayers embedded in a van der Waals heterostructure

classification cond-mat.mes-hall cond-mat.mtrl-sci
keywords diffusionexcitonexcitonsdarklengthneutralsamplesallowed
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We have combined spatially-resolved steady-state micro-photoluminescence ($\mu$PL) with time-resolved photoluminescence (TRPL) to investigate the exciton diffusion in a WSe$_2$ monolayer encapsulated with hexagonal boron nitride (hBN). At 300 K, we extract an exciton diffusion length $L_X= 0.36\pm 0.02 \; \mu$m and an exciton diffusion coefficient of $D_X=14.5 \pm 2\;\mbox{cm}^2$/s. This represents a nearly 10-fold increase in the effective mobility of excitons with respect to several previously reported values on nonencapsulated samples. At cryogenic temperatures, the high optical quality of these samples has allowed us to discriminate the diffusion of the different exciton species : bright and dark neutral excitons, as well as charged excitons. The longer lifetime of dark neutral excitons yields a larger diffusion length of $L_{X^D}=1.5\pm 0.02 \;\mu$m.

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