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Fermi velocity renormalization in graphene probed by terahertz time-domain spectroscopy

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arxiv 2006.00486 v1 pith:XRVOG4BM submitted 2020-05-31 cond-mat.mes-hall cond-mat.mtrl-sci

Fermi velocity renormalization in graphene probed by terahertz time-domain spectroscopy

classification cond-mat.mes-hall cond-mat.mtrl-sci
keywords graphenecarrierfermirenormalizationsubstrateselectricalfilmslarge-scale
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We demonstrate terahertz time-domain spectroscopy (THz-TDS) to be an accurate, rapid and scalable method to probe the interaction-induced Fermi velocity renormalization {\nu}F^* of charge carriers in graphene. This allows the quantitative extraction of all electrical parameters (DC conductivity {\sigma}DC, carrier density n, and carrier mobility {\mu}) of large-scale graphene films placed on arbitrary substrates via THz-TDS. Particularly relevant are substrates with low relative permittivity (< 5) such as polymeric films, where notable renormalization effects are observed even at relatively large carrier densities (> 10^12 cm-2, Fermi level > 0.1 eV). From an application point of view, the ability to rapidly and non-destructively quantify and map the electrical ({\sigma}DC, n, {\mu}) and electronic ({\nu}F^* ) properties of large-scale graphene on generic substrates is key to utilize this material in applications such as metrology, flexible electronics as well as to monitor graphene transfers using polymers as handling layers.

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