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Honeycomb lattice in metal-rich chalcogenide Fe2Te

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arxiv 2110.06415 v1 pith:CMF3ZGYG submitted 2021-10-13 cond-mat.mtrl-sci cond-mat.supr-con

Honeycomb lattice in metal-rich chalcogenide Fe2Te

classification cond-mat.mtrl-sci cond-mat.supr-con
keywords fe2teelectronicbandschalcogenidegrowthhoneycombmetal-richproperties
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Two-dimensional honeycomb crystals have inspired intense research interest for their novel properties and great potential in electronics and optoelectronics. Here, through molecular beam epitaxy on SrTiO3(001), we report successful epitaxial growth of metal-rich chalcogenide Fe2Te, a honeycomb-structured film that has no direct bulk analogue, under Te-limited growth conditions. The structural morphology and electronic properties of Fe2Te are explored with scanning tunneling microscopy and angle resolved photoemission spectroscopy, which reveal electronic bands cross the Fermi level and nearly flat bands. Moreover, we find a weak interfacial interaction between Fe2Te and the underlying substrates, paving a newly developed alternative avenue for honeycomb-based electronic devices.

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