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arxiv 2304.09731 v2 pith:5K6TS7XF submitted 2023-04-19 cond-mat.mes-hall cond-mat.str-elquant-ph

Excitonic Mott insulator in a Bose-Fermi-Hubbard system of moir\'e rm{WS}₂/rm{WSe}₂ heterobilayer

classification cond-mat.mes-hall cond-mat.str-elquant-ph
keywords bosonicmodelfermionicbose-fermi-hubbardexcitonsheterobilayerhubbardinsulator
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Understanding the Hubbard model is crucial for investigating various quantum many-body states and its fermionic and bosonic versions have been largely realized separately. Recently, transition metal dichalcogenides heterobilayers have emerged as a promising platform for simulating the rich physics of the Hubbard model. In this work, we explore the interplay between fermionic and bosonic populations, using a $\rm{WS}_2$/$\rm{WSe}_2$ heterobilayer device that hosts this hybrid particle density. We independently tune the fermionic and bosonic populations by electronic doping and optical injection of electron-hole pairs, respectively. This enables us to form strongly interacting excitons that are manifested in a large energy gap in the photoluminescence spectrum. The incompressibility of excitons is further corroborated by measuring exciton diffusion, which remains constant upon increasing pumping intensity, as opposed to the expected behavior of a weakly interacting gas of bosons, suggesting the formation of a bosonic Mott insulator. We explain our observations using a two-band model including phase space filling. Our system provides a controllable approach to the exploration of quantum many-body effects in the generalized Bose-Fermi-Hubbard model.

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  1. Unveiling the Spin-Valley Structure of Dipolar Exciton Ladders in R-stacked WSe$_2$/WS$_2$ Moir\'e Heterobilayers

    cond-mat.mes-hall 2026-07 conditional novelty 6.0

    Helicity-resolved magneto-photoluminescence reveals that the unequal spacing of the dipolar exciton ladder in R-stacked WSe₂/WS₂ arises from triplet and singlet spin-valley two-exciton states, not simple occupation-nu...