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Effective Equilibrium Theory of Quantum Light-Matter Interaction in Cavities: Extended Systems and the Long Wavelength Approximation

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arxiv 2312.17374 v2 pith:E7IKFA7W submitted 2023-12-28 cond-mat.mes-hall physics.opticsquant-ph

classification cond-mat.mes-hallphysics.opticsquant-ph
keywords cavityeffectiveelectromagneticextendedfinitelight-mattersystemstheory
verification ladder T0 review T1 audit T2 compute T3 formal
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When light and matter interact strongly, the resulting hybrid system inherits properties from both constituents, allowing one to modify material behavior by engineering the surrounding electromagnetic environment. This concept underlies the emerging paradigm of cavity materials engineering, which aims at the control of material properties via tailored vacuum fluctuations of dark photonic environments. The theoretical description of such systems is challenging due to the combined complexity of extended electronic states and quantum electromagnetic fields. Here, we derive an effective, non-perturbative theory for low-dimensional crystals embedded in a Fabry-P\'erot resonator, within the long-wavelength limit. Our approach incorporates the multimode and dispersive nature of the cavity field and reduces it to an effective single-mode description by imposing the condition of negligible momentum transfer from light to matter. Importantly, the resulting effective mode is characterized by a finite mode volume-even in the limit of extended cavities-which is directly linked to realistic cavity parameters. This ensures that the light-matter coupling remains finite in bulk systems. By explicitly accounting for the finite reflectivity of cavity mirrors, our theory also avoids double counting the contribution from free-space light-matter coupling. Overall, our results provide a robust and realistic framework for describing cavity-matter interactions at the Hamiltonian level, incorporating the electromagnetic environment beyond the idealized perfect-mirror approximation.

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Cited by 4 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Cavity Control of Strongly Correlated Electrons Beyond Resonant Coupling

    quant-ph 2026-03 conditional novelty 7.0 of 10

    Off-resonant cavity control of magnetic exchange is governed by the frequency-integrated photonic density of states relative to free space, making surface plasmon cavities effective and Fabry-Pérot cavities ineffective.

  2. Linear-Response Quantum-Electrodynamical Density Functional Theory Based on Two-Component X2C Hamiltonians

    physics.chem-ph 2025-07 conditional novelty 6.0 of 10

    A two-component X2C linear-response QEDFT method is derived, validated against four-component references, and applied to 2D spectra of mercury porphyrin and collective coupling in an AuH chain.

  3. Multiple Photon Field-induced Topological States in Bulk HgTe

    cond-mat.mtrl-sci 2025-06 conditional novelty 6.0 of 10

    Cavity photon fields are predicted to turn bulk HgTe into nodal-line, Weyl, or topological insulator phases depending on polarization orientation and coupling strength.

  4. Cavity-QED-controlled two-dimensional Moir\'e Excitons without twisting

    cond-mat.mtrl-sci 2025-08 reject novelty 5.0 of 10

    Spatially structured cavities are proposed as a twist-free route to Moiré-like exciton confinement, with dark-cavity mass renormalization attributed to cavity-mediated exciton-exciton interactions.

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