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arxiv 2504.13287 v1 pith:UFMUDU4E submitted 2025-04-17 quant-ph physics.atom-phphysics.optics

Theory of quantum optics and optical coherence in high harmonic generation

classification quant-ph physics.atom-phphysics.optics
keywords quantumopticalcorrelationfieldharmoniccoherencecorrelationsfunctions
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Optical coherence encodes information about the correlations of the electromagnetic field. In combination with quantum optical approaches, it allows for the study of the correlations between photons. Since the pioneering papers of Glauber, studies of optical coherence have facilitated many fundamental insights into non-classical signatures of light emission processes, with wide applicability in modern quantum technologies. However, when it comes to the photon up-conversion process of high-order harmonic generation the description has focused on semi-classical methods for decades. In this work, we overcome this limitation and establish a quantum optical theory of field correlations for the process of high harmonic generation (HHG). In effect, we introduce the notion of optical coherence at the intersection of quantum optics and strong laser-driven processes, and obtain the harmonic field correlation functions. In particular, we focus on the first and second order field correlation, which allow to understand the origin of the classical properties of the HHG spectrum, and its departure into the quantum regime. Further, we develop the theory for two-time intensity correlation functions of the harmonic field, and demonstrate the onset of anti-bunching signatures in HHG. We study the correlation functions in the regime of a single, few and many emitters in atomic HHG, showing the transition from quantum to classical signatures in the correlations. Since the theory is generic, it can be extended to multi-time correlation functions of any order, and allows to consider the interaction of light with arbitrary material systems.

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Cited by 4 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score.

  1. Attosecond metrology of bright quantum light

    quant-ph 2026-07 conditional novelty 7.0

    Attosecond streaking of bright squeezed light produces distinct sub-cycle modulations that encode quantum field quadrature fluctuations, enabling squeezing certification beyond conventional tomography limits.

  2. Emergence of Gaussian entanglement and non-Gaussianity in high-harmonic generation driven by bright squeezed light

    quant-ph 2026-06 unverdicted novelty 7.0

    Bichromatic HHG with coherent drive at ω and perturbative BSV at 2ω yields multimode Gaussian entanglement in even harmonics, modeled as a collective squeezed mode over the harmonic manifold.

  3. Photon anti-bunching in high harmonic generation

    quant-ph 2026-06 unverdicted novelty 7.0

    Prediction of photon anti-bunching in HHG via the Heisenberg picture approach, claimed as the first theoretical single-photon non-classicality signature in HHG temporal correlations.

  4. Emergence of nonclassical radiation in strongly laser-driven quantum systems

    quant-ph 2025-12 unverdicted novelty 7.0

    Nonclassical radiation in strongly driven systems originates from nonlinear dependence of the electronic dipole on the light-mode coordinate, producing squeezing or Wigner negativity depending on the order of nonlinearity.