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arxiv 1411.2479 v2 pith:HF6DWAO7 submitted 2014-11-10 cond-mat.mes-hall cond-mat.mtrl-sci

Low carrier concentration crystals of the topological insulator Bi_(2-x)Sb_(x)Te_(3-y)Se_(y): a magnetotransport study

classification cond-mat.mes-hall cond-mat.mtrl-sci
keywords topologicalbstscarriercrystalsbulk-insulatingconcentrationhighinsulator
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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In 3D topological insulators achieving a genuine bulk-insulating state is an important research topic. Recently, the material system (Bi,Sb)$_{2}$(Te,Se)$_{3}$ (BSTS) has been proposed as a topological insulator with high resistivity and a low carrier concentration (Ren \textit{et al.} \cite{Ren2011}). Here we present a study to further refine the bulk-insulating properties of BSTS. We have synthesized Bi$_{2-x}$Sb${_x}$Te$_{3-y}$Se$_{y}$ single crystals with compositions around $x = 0.5$ and $y = 1.3$. Resistance and Hall effect measurements show high resistivity and record low bulk carrier density for the composition Bi$_{1.46}$Sb$_{0.54}$Te$_{1.7}$Se$_{1.3}$. The analysis of the resistance measured for crystals with different thicknesses within a parallel resistor model shows that the surface contribution to the electrical transport amounts to 97% when the sample thickness is reduced to $1 \mu$m. The magnetoconductance of exfoliated BSTS nanoflakes shows 2D weak antilocalization with $\alpha \simeq -1$ as expected for transport dominated by topological surface states.

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