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Giant anisotropic anomalous Hall effect in antiferromagnetic topological metal NdGaSi

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arxiv 2409.06250 v1 pith:HIP45LXM submitted 2024-09-10 cond-mat.mes-hall cond-mat.mtrl-sci

Giant anisotropic anomalous Hall effect in antiferromagnetic topological metal NdGaSi

classification cond-mat.mes-hall cond-mat.mtrl-sci
keywords magneticanomaloushallndgasianisotropicantiferromagneticcm-1direction
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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The interplay between magnetism and strong electron correlation in magnetic materials discerns a variety of intriguing topological features. Here, we report a systematic investigation of the magnetic, thermodynamic, and electrical transport properties in NdGaSi single crystals. The magnetic measurements reveal a magnetic ordering below T_N (11 K), with spins aligning antiferromagnetically in-plane, and it orders ferromagnetically (FM) out-of-plane. The longitudinal resistivity data and heat capacity exhibit a significant anomaly as a consequence of the magnetic ordering at TN. The magnetoresistance study shows significantly different behavior when measured along either direction, resulting from the complex nature of the magnetic structure, stemming from complete saturation of moments in one direction and subsequent spin flop transitions in the other. Remarkably, we have also noticed an unusual anisotropic anomalous Hall response. We have observed a giant anomalous Hall conductivity (AHC) of 1730 ohm-1 cm-1 and 490 ohm-1 cm-1 at 2 K, with B // [001] and B // [100], respectively. Our scaling analysis of AHC reveals that the anomalous Hall effect in the studied compound is dominated by the Berry phase-driven intrinsic mechanism. These astonishing findings in NdGaSi open up new possibilities for antiferromagnetic spintronics in rare-earth-based intermetallic compounds.

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