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Large unconventional anomalous Hall effect far above room temperature in epitaxial Fe₃Ga₄ films

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arxiv 2507.07434 v1 pith:LZOGKPRP submitted 2025-07-10 cond-mat.mtrl-sci cond-mat.mes-hallcond-mat.str-el

Large unconventional anomalous Hall effect far above room temperature in epitaxial Fe₃Ga₄ films

classification cond-mat.mtrl-sci cond-mat.mes-hallcond-mat.str-el
keywords magneticuaheroomtemperatureeffectepitaxialexhibitfilms
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Noncoplanar spin textures usually exhibit a finite scalar spin chirality (SSC) that can generate effective magnetic fields and lead to additional contributions to the Hall effect, namely topological or unconventional anomalous Hall effect (UAHE). Unlike topological spin textures (e.g., magnetic skyrmions), materials that exhibit fluctuation-driven SSC and UAHE are rare. So far, their realization has been limited to either low temperatures or high magnetic fields, both of which are unfavorable for practical applications. Identifying new materials that exhibit UAHE in a low magnetic field at room temperature is therefore essential. Here, we report the discovery of a large UAHE far above room temperature in epitaxial Fe$_3$Ga$_4$ films, where the fluctuation-driven SSC stems from the field-induced transverse-conical-spiral phase. Considering their epitaxial nature and the large UAHE stabilized at room temperature in a low magnetic field, Fe$_3$Ga$_4$ films represent an exciting, albeit rare, case of a promising candidate material for spintronic devices.

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