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Dynamic screening of quasiparticles in WS₂ monolayers

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arxiv 2204.02125 v2 pith:QTQEDDD3 submitted 2022-04-05 cond-mat.mes-hall cond-mat.mtrl-sci

Dynamic screening of quasiparticles in WS₂ monolayers

classification cond-mat.mes-hall cond-mat.mtrl-sci
keywords excitonscreeningdynamicdynamicsbandbindingbluebroadening
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We unravel the influence of quasiparticle screening in the non-equilibrium exciton dynamics of monolayer WS$_2$. We report pump photon energy-dependent exciton blue and red-shifts from time-resolved-reflectance contrast measurements. Based on a phenomenological model, we isolate the effective impact of excitons and free carriers on the renormalization of the quasi-free particle band gap, exciton binding energy and linewidth broadening. By this, our work does not only provide a comprehensive picture of the competing phenomena governing the exciton dynamics in WS$_2$ upon photoexcitation, but also demonstrates that exciton and carrier contributions to dynamic screening of the Coulomb interaction differ significantly.

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