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Two-Dimensional Antimony Oxide

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arxiv 1909.01204 v4 pith:SVZY4XGT submitted 2019-09-03 cond-mat.mtrl-sci cond-mat.mes-hall

Two-Dimensional Antimony Oxide

classification cond-mat.mtrl-sci cond-mat.mes-hall
keywords antimonyoxideantimonenedifferentpropertiesstructurestwo-dimensionalband
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Two-dimensional (2D) antimony, so-called antimonene, can form antimonene oxide when exposed to air. We present different types of single- and few-layer antimony oxide structures, based on density functional theory (DFT) calculations. Depending on stoichiometry and bonding type, these novel 2D layers have different structural stability and electronic properties, ranging from topological insulators to semiconductors with direct and indirect band gaps between 2.0 and 4.9 eV. We discuss their vibrational properties and Raman spectra for experimental identification of the predicted structures.

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