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Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride

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arxiv 2011.12224 v2 pith:TA2GJ53Z submitted 2020-11-24 physics.optics cond-mat.mes-hallquant-ph

Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride

classification physics.optics cond-mat.mes-hallquant-ph
keywords emissionwavelengthemittersquantummaterialsborondeviceshexagonal
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Single photon emitters (SPEs) in low-dimensional layered materials have recently gained a large interest owing to the auspicious perspectives of integration and extreme miniaturization offered by this class of materials. However, accurate control of both the spatial location and the emission wavelength of the quantum emitters is essentially lacking to date, thus hindering further technological steps towards scalable quantum photonic devices. Here, we evidence SPEs in high purity synthetic hexagonal boron nitride (hBN) that can be activated by an electron beam at chosen locations. SPE ensembles are generated with a spatial accuracy better than the cubed emission wavelength, thus opening the way to integration in optical microstructures. Stable and bright single photon emission is subsequently observed in the visible range up to room temperature upon non-resonant laser excitation. Moreover, the low-temperature emission wavelength is reproducible, with an ensemble distribution of width 3 meV, a statistical dispersion that is more than one order of magnitude lower than the narrowest wavelength spreads obtained in epitaxial hBN samples. Our findings constitute an essential step towards the realization of top-down integrated devices based on identical quantum emitters in 2D materials.

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