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Directing Monolayer Tungsten Disulfide Photoluminescence using a Bent Plasmonic Nanowire on a Mirror Cavity

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arxiv 2203.00391 v1 pith:VP7RYCXG submitted 2022-03-01 physics.optics cond-mat.mtrl-sciphysics.app-phquant-ph

Directing Monolayer Tungsten Disulfide Photoluminescence using a Bent Plasmonic Nanowire on a Mirror Cavity

classification physics.optics cond-mat.mtrl-sciphysics.app-phquant-ph
keywords cavityphotoluminescenceemissionmirrormonolayernanowireopticalantennas
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Designing directional optical antennas without compromising the field enhancement requires specially designed optical cavities. Herein, we report on the experimental observations of directional photoluminescence emission from a monolayer Tungsten Disulfide using a bent-plasmonic nanowire on a mirror cavity. The geometry provides field enhancement and directivity to photoluminescence by sandwiching the monolayer between an extended cavity formed by dropcasting bent silver nanowire and a gold mirror. We image the photoluminescence emission wavevectors by using the Fourier plane imaging technique. The cavity out-couples the emission in a narrow range of wavevectors with a radial and azimuthal spreading of only 11.0{\deg} and 25.1{\deg}, respectively. Furthermore, we performed three dimensional finite difference time domain based numerical calculations to corroborate and understand the experimental results. We envisage that the results presented here will be readily harnessed for on-chip coupling applications and in designing inelastic optical antennas.

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