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Transient grating spectroscopy on a DyCo₅ thin film with femtosecond extreme ultraviolet pulses

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arxiv 2311.01399 v2 pith:ZPEVXNPN submitted 2023-11-02 cond-mat.mtrl-sci cond-mat.mes-hall

Transient grating spectroscopy on a DyCo₅ thin film with femtosecond extreme ultraviolet pulses

classification cond-mat.mtrl-sci cond-mat.mes-hall
keywords pulsestransientdycodynamicsexcitedextremefemtosecondfilm
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Surface acoustic waves (SAWs) are excited by femtosecond extreme ultraviolet (EUV) transient gratings (TGs) in a room-temperature ferrimagnetic DyCo$_5$ alloy. TGs are generated by crossing a pair of EUV pulses from a free electron laser (FEL) with the wavelength of 20.8\,nm matching the Co $M$-edge, resulting in a SAW wavelength of $\Lambda=44$\,nm. Using the pump-probe transient grating scheme in a reflection geometry the excited SAWs could be followed in the time range of -10 to 100\,ps in the thin film. Coherent generation of TGs by ultrafast EUV pulses allows to excite SAW in any material and to investigate their couplings to other dynamics such as spin waves and orbital dynamics. In contrast, we encountered challenges in detecting electronic and magnetic signals, potentially due to the dominance of the larger SAW signal and the weakened reflection signal from underlying layers. A potential solution for the latter challenge involves employing soft X-ray probes, albeit introducing additional complexities associated with the required grazing incidence geometry.

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