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Propagating Collective Spin-valley Modes in Twisted WSe2

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arxiv 2507.18770 v2 pith:PVLTG675 submitted 2025-07-24 cond-mat.mes-hall cond-mat.str-elquant-ph

Propagating Collective Spin-valley Modes in Twisted WSe2

classification cond-mat.mes-hall cond-mat.str-elquant-ph
keywords modemodesneutralcollectivegoldstonespin-valleystatetwisted
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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The emergence of neutral collective modes is a hallmark of correlated quantum phases but is often challenging to probe experimentally. In two-dimensional flatband systems, charge responses have been intensively investigated yet neutral excitations remain largely unexplored. In particular, intervalley coherent state (IVC) features a neutral Goldstone mode due to spontaneously broken valley U(1) symmetry. While IVC state has been proposed as a unifying theme across graphene and semiconductor based systems, its defining feature, the neutral Goldstone mode, remains elusive in experiment. Here we investigate space and time resolved transport of neutral modes in twisted WSe2 moire superlattices through a novel ultrafast imaging technique. We uncover two new propagating collective modes with very different velocities, which emerge near the van Hove singularity (VHS) in both intermediate (3.5 to 4 degree) and large (around 5 degree) angle twisted WSe2. The fast-propagating mode has a large speed of about 3 km/s and is consistent with a Goldstone mode for an IVC state, while the slow-moving mode is likely a gapped amplitude mode. They can be understood as the spin-valley analogues of collective modes of a superfluid, whose propagation is imaged for the first time in a condensed matter system. Our study demonstrates a powerful new approach for probing charge-neutral modes in quantum materials and offers key insights into the interplay between charge and spin-valley physics in moire superlattices.

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  1. Multi-Q spin-valley order in twisted WSe2

    cond-mat.str-el 2025-10 conditional novelty 7.0

    At ν=1 in 3.65°-twisted WSe2, Hartree-Fock predicts that the 120° antiferromagnet gives way to coplanar or non-coplanar multi-Q magnetic order with four ordering wavevectors and soft M-point spin fluctuations.