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Results of a search for a long-range monopole-dipole coupling between the mass of the Earth and rubidium (Rb) nuclear spins are reported. The experiment simultaneously measures the spin precession frequencies of overlapping ensembles of $^{85}$Rb and $^{87}$Rb atoms contained within an evacuated, antirelaxation-coated vapor cell. The nuclear structure of the Rb isotopes makes the experiment particularly sensitive to spin-dependent interactions of the proton. The spin-dependent component of the gravitational energy of the proton in the Earth's field is found to be smaller than $3 \times 10^{-18}~{\rm eV}$, improving laboratory constraints on long-range monopole-dipole interactions by over three orders of magnitude.