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Observation of Giant Spin Splitting and d-wave Spin Texture in Room Temperature Altermagnet RuO2

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arxiv 2402.04995 v1 pith:MBMQLFMT submitted 2024-02-07 cond-mat.mtrl-sci cond-mat.other

Observation of Giant Spin Splitting and d-wave Spin Texture in Room Temperature Altermagnet RuO2

classification cond-mat.mtrl-sci cond-mat.other
keywords spind-wavephaseroomruo2temperaturealtermagnetsplitting
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Recently, a novel magnetic phase called altermagnetism has been proposed, ushering in a third distinct magnetic phase beyond ferromagnetism and antiferromagnetism. It is expected that this groundbreaking phase exhibits unique physical properties such as C-paired spin-valley locking, anomalous Hall effect, nontrivial Berry phase, and giant magnetoresistance, etc. Among all the predicted candidates, several room temperature altermagnets are suggested to host significant potential applications in the near future. Nevertheless, direct evidence about the spin pattern of the room temperature altermagnet is still unrevealed. Previous studies found that RuO2 is identified as the most promising candidate for room temperature d-wave altermagnetism, exhibiting a substantial spin splitting of up to 1.4 eV. In this study, utilizing angle-resolved photoemission spectroscopy (ARPES), we report experimental observation of the spin splitting in RuO2. Furthermore, employing spin-ARPES, we directly observed the d-wave spin pattern. Our results unequivocally show that RuO2 is a perfect d-wave altermagnet with great potential for upcoming spintronic applications.

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Cited by 11 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score.

  1. Intrinsic antiferromagnetic half-metal and topological phases from the ferrovalley states of the sliding bilayer altermagnets

    cond-mat.mtrl-sci 2025-09 conditional novelty 7.0

    Sliding bilayer altermagnets host antiferromagnetic half-metallicity and Chern insulator phases via spin-dependent interlayer hopping in ferrovalley states, demonstrated in V2OSSe by first-principles calculations.

  2. Orbital-Selective Mott Transition and Correlation-Amplified Charge Ordering in the Altermagnet CsCr$_2$S$_2$O

    cond-mat.str-el 2026-07 conditional novelty 6.0

    Dynamical correlations amplify S-distortion-seeded dyz charge asymmetry between Cr sites, driving the Verwey-type MIT in altermagnetic CsCr2S2O; Te substitution is predicted to suppress it.

  3. Giant Room-Temperature Third-Order Electrical Transport in a Thin-Film Altermagnet Candidate

    cond-mat.mes-hall 2026-04 unverdicted novelty 6.0

    Giant room-temperature third-order Hall effect observed in RuO2 thin films is correlated with altermagnetic order via quantum geometry.

  4. Superconducting States and Intertwined Orders in Metallic Altermagnets

    cond-mat.supr-con 2026-03 conditional novelty 6.0

    In C4T-symmetric d-wave altermagnets, equal-spin p-wave pairing condenses in two non-degenerate two-component gap sets, producing two transition temperatures, with nematic and spin-current-loop fluctuations respective...

  5. Tunneling magnetoresistance in a junction made of $X$-wave magnets with $X=p,d,f,g,i$

    cond-mat.mes-hall 2025-09 unverdicted novelty 6.0

    A universal analytic formula for the TMR ratio in X-wave magnet junctions is derived, proportional to |J|/(N_X Γ) for small Γ, in contrast to the J²/Γ² dependence for ferromagnets.

  6. Global magnetic phase diagram and multiple unconventional magnets in NiAs-type compounds

    cond-mat.mtrl-sci 2026-05 unverdicted novelty 5.0

    A J1-J2-J3 Heisenberg model plus DFT yields a global phase diagram for NiAs-type compounds that includes new g-wave altermagnets, f-wave OPMs, and mixed-parity states dominated by f-wave in CrSe and CrTe1-xSex.

  7. Nonmagnetic-magnetic Transitions in Rutile RuO2

    cond-mat.mtrl-sci 2026-04 unverdicted novelty 5.0

    DFT calculations show RuO2 undergoes transitions between nonmagnetic and altermagnetic ground states as a function of Hubbard U and strain that changes cell volume.

  8. Nonmagnetic-magnetic Transitions in Rutile RuO2

    cond-mat.mtrl-sci 2026-04 conditional novelty 5.0

    Correlation strength and volume-changing strain can switch bulk rutile RuO2 between nonmagnetic and multiple altermagnetic phases with spin splitting.

  9. Incipient magnetic instability in RuO$_2$ with random phase approximation

    cond-mat.mtrl-sci 2026-03 unverdicted novelty 5.0

    RuO2 exhibits a leading instability toward commensurate altermagnetic order at low temperatures in the stoichiometric non-magnetic phase according to RPA analysis of susceptibility.

  10. Fermi-liquid behavior and characteristic temperature-dependent susceptibility in clean RuO$_2$ crystal

    cond-mat.mtrl-sci 2025-12 unverdicted novelty 4.0

    Ultra-clean RuO2 crystals exhibit weakly correlated 3D Fermi-liquid behavior with susceptibility increasing with temperature due to lattice-expansion effects on the band structure.

  11. Growth of ultra-clean single crystals of RuO2

    cond-mat.str-el 2025-05 accept novelty 4.0

    Ultra-clean RuO2 single crystals grown via necked-tube sublimation transport achieve RRR up to 1200 with residual resistivity around 30 nOhm cm and no detected magnetic order.